By Chunshan Song, Anne F. Gaffney, and Kaoru Fujimoto (Eds.)
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ACS Symposium Series; American Chemical Society: Washington, DC, 2002. 52 W. Hoelderich, German Patent DE 98-19845975 X. Longya, L. Liwu, W. Qingxia, Y. Li, W. Weichen, NATURAL GAS CONVERSION V. Studies in Surface Science and Catalysis, Vol. 119, 605-610 (1998), A. Parmaliana et al (Editors) Elsevier Science Β. V. 4, 1987 S. Wang, K. Murata, T. Hayakawa, S. Hamakawa, K. ; ACS Symposium Series; American Chemical Society: Washington, DC, 2002.
The Mars-van Krevelen mechanism suggests that a gain in selectivity is possible by keeping the gas phase oxygen from the process. The lattice oxygen of the catalyst is used in a stoichiometric reaction with a hydrocarbon to yield the oxygenated product. The reduced oxide catalyst is then transported to a separate zone and re-oxidized by air. The process is referred to as anaerobic oxidation. For this complex engineering and catalysis to be successful and economically viable, several requirements must be met.
Oyama, A. M. Gaffney and J. JE. Lyons (Editors), V o l . 110, 847-856, 1 9 9 7 , Elsevier Science Β. V . A . K . Uriarte, M. A . Rodkin, M. J. Gross, A . S. Kharitonov and G . I. Panov, 3 World Congress on Oxidation Catalysis, R. K . Grasselli, S. T. Oyama, A. M. Gaffney and J. JE. Lyons (Editors), Vol. 110, 857-864, 1 9 9 7 , Elsevier Science Β. V . M. G. Clerici, Heterogeneous Catalysis and Fine Chemicals III, 21-33 (1993), M. Guisnet et al (Editors) Elsevier Science Publishers Β. V . 20 L . W .